Journal
RSC ADVANCES
Volume 10, Issue 56, Pages 33972-34005Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0ra05858k
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Funding
- National Natural Science Foundation of China [21666008, 21908033, 21576059]
- Fok Ying-Tong Education Foundation [161030]
- Guizhou Science & Technology Foundation [[2018]1037]
- Program of Introducing Talents of Discipline to Universities of China (111 Program) [D20023]
- Chinese State Scholarship [201906670009]
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Carbon dioxide is an ideal raw material for the synthesis of complex organic compounds because of its rich, non-toxic, and good physical properties. It is of great significance to transform CO(2)into valuable fine chemicals and develop a green sustainable cycle of carbon surplus. Based on hydrosilane as a reducing agent, this work summarizes the recent applications of reductive amidation of CO(2)using different catalysts such as organocatalysts, ionic liquids (ILs), salts, transition metal complexes, and solvents. The main factors affecting the reductive amidation of CO(2)and the possible reaction mechanism are discussed. Moreover, the future orientation and catalytic systems of the formylation of amines with CO(2)and hydrosilane are prospected.
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