4.6 Article

Effective removal of particulate matter from air by using zeolite-coated filters

Journal

JOURNAL OF MATERIALS CHEMISTRY A
Volume 8, Issue 35, Pages 17960-17968

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/d0ta04914j

Keywords

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Funding

  1. Basic Science Research Program through the National Research Foundation of Korea (NRF) - Ministry of Science, ICT and future Planning [2017R1A2B2008774]
  2. National Research Foundation of Korea [4120200213748] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)

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Removal of particulate matter (PM) from air is very important for a safe environment and sound health. In this work, we first applied zeolites, after coating onto substrates such as cotton and polyester, in PM removal from air and confirmed that zeolites, especially aluminous ones, could be very effective in the removal of PM. For example, NaX/cotton (NaX: similar to 20 wt% of cotton) showed 3.6- and 3.4-times the removal efficiency (RE) of bare cotton for PM2.5 and PM10 elimination, respectively, even though the pressure drop increased only slightly (by 9 Pa). Moreover, NaX was much more effective than the widely applied metal-organic frameworks (MOFs) such as ZIF-8, UiO-66 and MOF-74 (or CPO-27), even though the porosity of NaX was much lower than those of the applied MOFs. Importantly, the quality factor and RE of the filters increased linearly with the increasing Al contents of the applied zeolites (with the same faujasite structure, namely NaY and NaX), suggesting the important role of Al and charge-compensating Na+ in PM elimination from air. Finally, it could be suggested that the PM removal is due to electrostatic interactions and aluminous zeolites (with charge-balancing cations) can be effectively used in the PM removal from air.

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