Journal
CHEMICAL SOCIETY REVIEWS
Volume 49, Issue 18, Pages 6555-6567Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c9cs00541b
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Funding
- Research Grants Council of the Hong Kong Special Administrative Region, China [14201317, 14207419, 14210517, N-CUHK407/16, AoE/P-0/12]
- VC Discretionary Fund by the Chinese University of Hong Kong [8601014]
- National Research Foundation Singapore [NRF2017-NRF-ANR002 2DPS]
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Liquid-liquid droplet reactors have garnered significant interest in biochemical applications with the obvious benefits of reduced reagent consumption, well controlled droplet size and confinement of biochemical reactions away from external interference. This Tutorial Review provides a succinct overview of widely employed liquid-liquid droplet reactors, namely single emulsions, multiple emulsions and all-aqueous emulsions, under the scope of thermodynamics, with a particular emphasis on how their intrinsic interfacial properties may endow mass transport for a variety of demands. Beyond spatially compartmentalizing a thermodynamic system, the artificial interface of droplet reactors has shown initial promising for multi-step or complex reactions. Moving forward, the artificial interface shall be tailored further towards functional to imitate the intelligent interface surrounding natural vesicles or cells.
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