Journal
INFOMAT
Volume 2, Issue 6, Pages 1057-1076Publisher
WILEY
DOI: 10.1002/inf2.12118
Keywords
electrocatalysis; electrochemical energy storage; interlayer space; MXene; structure design
Categories
Funding
- Zhejiang University of Technology
- Natural Science Foundation of Zhejiang Province [LD18E020003]
- National Natural Science Foundation of China [51722210]
- Dartmouth College
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2D transition metal carbides, carbonitrides, and nitrides known as MXenes possess high electrical conductivity, large redox active surface area, rich surface chemistry, and tunable structures. Benefiting from these exceptional chemical and physical properties, the applications of MXenes for electrochemical energy storage and conversion have attracted increasing research interests around the world. Notably, the electrochemical performances of MXenes are directly dependent on their synthesis conditions, interfacial chemistries and structural configurations. In this review, we summarize the synthesis techniques of MXenes, as well as the recent advances in the interfacial structure design of MXene-based nanomaterials for electrochemical energy storage and conversion applications. Additionally, we provide an in-depth discussion on the relationship between interfacial structure and electrochemical performance from the perspectives of energy storage and electrocatalysis mechanisms. Finally, the challenges and insights for the future research of interfacial structure design of MXenes are outlined.
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