Journal
CHEMICAL COMMUNICATIONS
Volume 56, Issue 80, Pages 11945-11948Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0cc04274a
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Funding
- Japan Society for the Promotion of Science (JSPS) [JP19H02735]
- Cooperative Research Program of Dynamic Alliance for Open Innovation Bridging Human, Environment and Materials'' [20193019, 20203024]
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A B-12 complex-BODIPY dyad was synthesized by peripheral modification of cobalamin derivatives. The photophysical properties of the dyad were investigated by UV-vis, PL, and transient absorption spectroscopy. A visible light-driven dechlorination reaction of a trichlorinated organic compound, DDT, was reported. The dyad showed efficient catalysis for dechlorination under N-2 with turnover numbers of over 220 for the reaction. One-pot syntheses of an ester and amide from DDT and benzotrichloride were also achieved using the dyad under air.
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