Journal
CHEMICAL COMMUNICATIONS
Volume 56, Issue 84, Pages 12817-12820Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0cc05271j
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Funding
- National Natural Science Foundation of China [21778025, 21762021]
- Science and Technology Project of Jiangxi Provincial Education Department [GJJ150297]
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A facile approach to the fully substituted cyclopentenones involving an unprecedented benzofuran-ring-opening is described. The cleavage of a benzofuran endocyclic C2-O bond proceeded smoothly in the absence of any transition metal catalyst or highly reactive organometallic reagent. Such benzofuran-ring-opening is delicately incorporated into an acid-catalyzed cascade process, orchestrating a novel synthetic strategy for complex cyclopentenones with excellent yields and diastereoselectivities.
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