Journal
CHEMICAL ENGINEERING JOURNAL
Volume 400, Issue -, Pages -Publisher
ELSEVIER SCIENCE SA
DOI: 10.1016/j.cej.2020.125843
Keywords
Zn metal anode; Li metal anode; Dendrite-free; 3D carbon; Heteroatom-doped
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Funding
- National Natural Science Foundation of China [51871135]
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The cycling life of rechargeable metal cells is mainly restricted by dendritic growth of metals. Herein, N/O dual-doped 3D porous carbon architectures are designed on commercial Cu foam current collector (NOCA@CF) from MOF arrays precursors to suppress the dendrite growth of metal anodes. The unique architecture provides integrated merits of good hydrophilicity/lithiophilicity, abundant nuclear sites, high electronic conductivity and robust framework, which can significantly suppress the dendrite growth of both the aqueous zinc metal anode and nonaqueous lithium metal anode. As a result, both aqueous Zn@NOCA@CF parallel to ILiMn2O4 full cells and non-aqueous Li@NOCA@CF parallel to LiNi0.5Mn1.5O4, Li@NOCA@CF parallel to LiNi0.8Co0.1Mn0.1O2 full cells show superior stable electrochemical performance with high rate capability. Moreover, the results may be interesting for researchers on other metal based rechargeable batteries.
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