4.8 Article

Nanoscale Conductivity Imaging of Correlated Electronic States in WSe2/WS2 Moire Superlattices

Journal

PHYSICAL REVIEW LETTERS
Volume 125, Issue 18, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.125.186803

Keywords

-

Funding

  1. U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences [DE-SC0019025]
  2. Welch Foundation [F-1814]
  3. Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division of the U.S. Department of Energy [DE-AC02-05CH11231, KCWF16]
  4. U.S. Army Research Office under MURI [W911NF-17-1-0312]
  5. Elemental Strategy Initiative by the MEXT, Japan [JPMXP0112101001]
  6. JSPS KAKENHI [JP20H00354]
  7. CREST, JST [JPMJCR15F3]
  8. NSF [DMR 1552220, DMR 1904716, CMMI 1933214]
  9. Department of Defense (DoD) through the National Defense Science & Engineering Graduate Fellowship (NDSEG) Program
  10. [DOE-SC0020653]
  11. U.S. Department of Energy (DOE) [DE-SC0019025] Funding Source: U.S. Department of Energy (DOE)

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We report the nanoscale conductivity imaging of correlated electronic states in angle-aligned WSe2/WS2 heterostructures using microwave impedance microscopy. The noncontact microwave probe allows us to observe the Mott insulating state with one hole per moire unit cell that persists for temperatures up to 150 K, consistent with other characterization techniques. In addition, we identify for the first time a Mott insulating state at one electron per moire unit cell. Appreciable inhomogeneity of the correlated states is directly visualized in the heterobilayer region, indicative of local disorders in the moire superlattice potential or electrostatic doping. Our work provides important insights on 2D moire systems down to the microscopic level.

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