Journal
NEW JOURNAL OF CHEMISTRY
Volume 44, Issue 44, Pages 19184-19191Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0nj04085a
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Funding
- Analysis and Testing Center of Nanjing University of Science and Technology
- National Special Superfine Powder Engineering Technology Research Center
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The problem of debonding the interface between propellant grain and propellant coating has been a tricky problem that has puzzled many scholars. Self-healing adhesives are expected to solve this problem. Herein, we studied the most widely used HTPB system in composite propellants. By adopting free radical polymerized HTPB as the soft segment of the adhesive and introducing aromatic disulfides, we successfully prepared a self-healing polyurethane adhesive. The adhesive can self-heal at a safe temperature of 80 degrees C, with an elongation at break of more than 700% and a self-healing efficiency of up to 97%, and has excellent thermal stability. The interface self-healing experiment showed that the adhesive can recover the debonding damage at the interface. Our results will provide a new insight into the rebonding of the interface between propellant grain and coating.
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