4.7 Article

Fabrication of MoS2QDs/ZnO nanosheet 0D/2D heterojunction photocatalysts for organic dyes and gaseous heavy metal removal

Journal

JOURNAL OF COLLOID AND INTERFACE SCIENCE
Volume 579, Issue -, Pages 853-861

Publisher

ACADEMIC PRESS INC ELSEVIER SCIENCE
DOI: 10.1016/j.jcis.2020.06.116

Keywords

OD/2D heterojunction; MoS2 QDs; ZnO nanosheets; RhB degradation; Elemental mercury removal

Funding

  1. National Natural Science Foundation of China [51864030, 51522405]
  2. National Key R&D Program of China [2018YFC1901904]
  3. Yunnan Provincial Science and Technology Talents Program [2019HB003]
  4. Yunnan Science and Technology Major Project [2018ZE008, 2018ZE027]
  5. Kunming University of Science and Technology [KKZ3201752046, KKSY201732033]
  6. Yunnan Education Department [2019 J0034]
  7. Analysis and Testing Foundation of Kunming University of Science and Technology [2018T20110222]
  8. Yunnan Provincial Youth Top-notch Talent Support Program

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In this paper, a novel 0D/2D heterojunction photocatalyst based on MoS2 QDs/ZnO nanosheets was successfully constructed by a simple two-step process, and its photocatalytic behavior for organic dyes (RhB) degradation and gaseous heavy metals (Hg) removal under ultraviolet light were studied. For the optimum 5% MoS2/ZnO photocatalyst, 95% of RhB could be removed in 50 min, and 99.8% of the gaseous mercury could be removed in 60 min. Besides, MoS2 QDs/ZnO nanosheets also exhibited excellent photocatalytic durability. The constructed 0D/2D heterojunctions could efficiently improve the separation efficiency and charge transfer of photogenerated carriers, thus improving the photocatalytic activity. Therefore, this strategy provided a new way to design bifunctional 0D/2D heterojunction photocatalysts for water treatment and air pollution. (C) 2020 Elsevier Inc. All rights reserved.

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