Journal
DALTON TRANSACTIONS
Volume 49, Issue 44, Pages 15587-15591Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0dt03205k
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Funding
- Hong Kong General Research Fund [HKBU12304320]
- Hong Kong Baptist University [FRG2-17-18-068, RC-ICRS/15-16/02E, RC-ICRS/1617/02C-CHE, RC-ICRS-18-19-01A, RC-IRMS/16/17/02CHEM]
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Donor-acceptor two-dimensional covalent organic frameworks, PD-COF-23 and PD-COF-23-Ni, are constructed and applied for selective CO2 reduction with CO conversion rates of 20.9 mu mol g(-1) h(-1) and 40.0 mu mol g(-1) h(-1), respectively, in the absence of any additional photosensitizers and noble metal co-catalysts within an operation time of 25 h. The multilayer nanosheet structure, efficient charge separation and transport, and internal reductive quenching cycle of the NiTAPP fragments of PD-COF-23-Ni result in its higher photocatalytic efficiency than that of PD-COF-23.
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