Journal
JOURNAL OF MATERIALS CHEMISTRY C
Volume 8, Issue 46, Pages 16418-16426Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0tc00622j
Keywords
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Funding
- National Natural Science Foundation of China [51772177]
- Shaanxi Science & Technology Co-ordination & Innovation Project of China [2017TSCXL-GY-08-05]
- Science Fund for Distinguished Young Scholars of Shaanxi Province [2018JC-029]
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Porous carbon-based composites have attracted extensive attention because of their good performance. However, designing and synthesizing porous carbon-based composites with excellent electromagnetic wave attenuation capabilities is still a great challenge. Herein, metal-organic frameworks act as good precursors, which can be used to prepare the hierarchical layered double hydroxide@carbon (LDH@C) composites using a facile three-step method. In this work, through the synergetic effects between the layered structure of the double hydroxide (LDH) and porous carbon, the hierarchical LDH@C composites achieved substantially strong electromagnetic wave absorption properties and a broad bandwidth. Furthermore, the hierarchical LDH@C composites with internal void space obtained by adjusting the Co/Al ratio can promote the multiple reflections of electromagnetic waves. As a result, the hierarchical LDH@C composites exhibit highly efficient electromagnetic wave absorption capabilities by adjusting their loading to 20 wt%. Specifically, the maximum reflection loss (RL) of the hierarchical LDH@C composites at 11.36 GHz is -64.8 dB, and the effective absorption bandwidth (RL <= -10 dB) of 9.0 GHz can be achieved. The results imply that the microwave absorption properties of the hierarchical LDH@C composites show a broad bandwidth and strong absorption.
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