Journal
RSC ADVANCES
Volume 10, Issue 63, Pages 38478-38483Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0ra07698h
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Funding
- National Natural Science Foundation of China [21801087]
- Fundamental Research Funds for the Central Universities CCNU [CCNU19QN064]
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A highly enantioselective copper-catalyzed propargylic amination starting from benzylic allylic amines has been developed with a new chiral N,N,P ligand. A series of N-tethered 1,6-enynes were synthesized in good to excellent yields with excellent enantioselectivities. Utilization of transition metal-catalyzed cycloisomerization of 1,6-enynes provides several enantioselectively enriched chiral five-membered N-heterocycles efficiently.
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