Journal
CHEMICAL COMMUNICATIONS
Volume 56, Issue 93, Pages 14677-14680Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0cc06492k
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Funding
- National Natural Science Foundation of China [91945301]
- National Key R&D Program of China [2017YFB0602202]
- Program of Shanghai Academic/Technology Research Leader [20XD1404000]
- Key Research Program of Frontier Sciences of the Chinese Academy of Sciences [QYZDB-SSW-SLH035]
- ''Transformational Technologies for Clean Energy and Demonstration'' of CAS [XDA21020600]
- Strategic Priority Research Program of CAS [XDA21020600]
- Youth Innovation Promotion Association of CAS
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Cu single atoms embedded in the C3N4 (Cu-SAs/C3N4) matrix exhibited high activity with 95% oxygenate selectivity for the direct conversion of methane at ambient temperature. The presence of abundant anchoring sites in C3N4 led to highly dispersed Cu-N-4 moieties, which were suggested to be the underlying active sites for methane conversion.
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