Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 85, Issue 23, Pages 15072-15081Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.0c01957
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Funding
- EU [SEP 210165479]
- FET open project QuIET [767187]
- Swiss National Science Foundation (SNF) [200020-178808]
- Fondecyt Regular Project [1181080]
- 111 project [90002-18011002]
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Porphyrin cydophane 1, consisting of two rigidly fixed but still movable cofacial porphyrins and exposing acetate-masked thiols in opposed directions of the macrocycle, is designed, synthesized, and characterized. The functional cyclophane 1, as pioneer of mechanosensitive 3D materials, forms stable single-molecule junctions in a mechanically controlled break-junction setup. Its reliable integration in a single-molecule junction is a fundamental prerequisite to explore the potential of these structures as mechanically triggered functional units and devices.
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