Journal
ORGANIC LETTERS
Volume 22, Issue 21, Pages 8702-8707Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.0c03294
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Funding
- National Natural Science Foundation of China [21772094, 21977049]
- Natural Science Foundation of Jiangsu Province [BK20191306]
- Program of Introducing Talents to Chinese Universities (111 Program) [D20023]
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Drimane meroterpenoids have attracted an increasing amount of attention in the discovery of therapeutically important probes, while the laggard synthetic accessibility is a conspicuous challenge. A new paradigm merging decarboxylative borylation and Suzuki coupling was developed as a powerful platform. Key features include the mild conditions, good chemoselectivity, operational facility, scalability, and easy availability of the coupling partners. This practical strategy enables the expedient formal synthesis of a large number of natural products and rapid generation of analogues.
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