4.8 Article

High-Throughput Electrical Characterization of Nanomaterials from Room to Cryogenic Temperatures

Journal

ACS NANO
Volume 14, Issue 11, Pages 15293-15305

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsnano.0c05622

Keywords

nanoelectronic device arrays; scalable fabrication; high-throughput testing; graphene and 2D materials; nanowires; electronic characterization

Funding

  1. Engineering and Physical Sciences Research Council [EP/R029075/1]
  2. Royal Commission for the Exhibition of 1851
  3. Royal Society Dorothy Hodgkin Research Fellowship
  4. EPSRC [EP/P005152/1]
  5. EPSRC Doctoral Training Award [EP/M508007/1]
  6. Australian Research Council
  7. European Commission [828841]
  8. UK's EPSRC [EP/N509760, EP/R03480X/1, EP/P013597/1]
  9. Ministry of Science and Technology (Taiwan)
  10. EPSRC [EP/P005152/1, EP/P013597/1, EP/R029075/1, EP/S019324/1, EP/R03480X/1] Funding Source: UKRI

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We present multiplexer methodology and hardware for nanoelectronic device characterization. This high-throughput and scalable approach to testing large arrays of nanodevices operates from room temperature to milli-Kelvin temperatures and is universally compatible with different materials and integration techniques. We demonstrate the applicability of our approach on two archetypal nanomaterials-graphene and semiconductor nanowires-integrated with a GaAs-based multiplexer using wet or dry transfer methods. A graphene film grown by chemical vapor deposition is transferred and patterned into an array of individual devices, achieving 94% yield. Device performance is evaluated using data fitting methods to obtain electrical transport metrics, showing mobilities comparable to nonmultiplexed devices fabricated on oxide substrates using wet transfer techniques. Separate arrays of indium-arsenide nanowires and micromechanically exfoliated monolayer graphene flakes are transferred using pick-and-place techniques. For the nanowire array mean values for mobility mu(FE) = 880/3180 cm(2) V-1 s(-1) (lower/upper bound), subthreshold swing 430 mV dec(-1), and on/off ratio 3.1 decades are extracted, similar to nonmultiplexed devices. In another array, eight mechanically exfoliated graphene flakes are transferred using techniques compatible with fabrication of two-dimensional superlattices, with 75% yield. Our results are a proof-of-concept demonstration of a versatile platform for scalable fabrication and cryogenic characterization of nanomaterial device arrays, which is compatible with a broad range of nanomaterials, transfer techniques, and device integration strategies from the forefront of quantum technology research.

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