Journal
GREEN CHEMISTRY
Volume 19, Issue 11, Pages 2653-2665Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7gc00491e
Keywords
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Funding
- CPER Structuration du Pole de Competitivite Fibres Grand'Est (Competitiveness Fibre Cluster), through local (Conseil General des Vosges)
- regional (Region Lorraine)
- national (DRRT)
- national (FNADT)
- European (FEDER) funds
- CHEERS project (FEDER funds)
- University of Lorraine
- Region Lorraine
- CNRS
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Highly N- and O-doped carbons were prepared from pine tannins by hydrothermal carbonisation (HTC) and subsequently applied as materials for supercapacitor electrodes. Pine tannins were transformed into carbon materials by using environment-friendly solvents (water or ammonia) without applying any activation or functionalisation post-treatment. Depending on the solution used for extracting tannins and on the HTC method, carbons with different physicochemical and electrochemical properties were obtained. The material prepared from the water-extracted tannin and subjected to HTC in ammonia displayed a porous texture composed of: (a) low ultramicroporosity and well-developed mesoporosity; (b) a hydrophilic surface with a high density of surface functionalities; and (c) a high nanotextural order. These features accounted for the excellent electrochemical performance of the resultant carbon electrode in terms of high rate capability up to 1 V s(-1), high energy density up to similar to 1500 mA g(-1), low cell resistance and fast frequency response, making it a suitable material for practical supercapacitors.
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