4.2 Article

Interaction of edge exciton polaritons with engineered defects in the hyperbolic material Bi2Se3

Journal

COMMUNICATIONS MATERIALS
Volume 2, Issue 1, Pages -

Publisher

SPRINGERNATURE
DOI: 10.1038/s43246-020-00108-9

Keywords

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Funding

  1. European Research Council (ERC starting Grant NanoBeam)
  2. European Research Council (ERC Advanced Grant ComplexPlas)
  3. Bundesministerium fur Bildung und Forschung
  4. Deutsche Forschungsgemeinschaft [SPP1839]
  5. Baden-Wurttemberg Stiftung
  6. European Union's Horizon 2020 research and innovation program [823717 - ESTEEM3]

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This study investigates the hyperbolic optical properties of Bi2Se3 material, demonstrating the support for exciton polaritons. The research compares the behavior of polaritons propagating along edges in pristine and artificially structured conditions, confirming the ability to control the direction of edge polariton propagation through structural manipulation.
Hyperbolic materials exhibit unique properties that enable intriguing applications in nanophotonics. The topological insulator Bi2Se3 represents a natural hyperbolic optical medium, both in the THz and visible range. Here, using cathodoluminescence spectroscopy and electron energy-loss spectroscopy, we demonstrate that Bi2Se3 supports room-temperature exciton polaritons and explore the behavior of hyperbolic edge exciton polaritons, which are hybrid modes resulting from the coupling of the polaritons bound to the upper and lower edges of Bi2Se3 nanoplatelets. We compare Fabry-Perot-like resonances emerging in edge polariton propagation along pristine and artificially structured edges and experimentally demonstrate the possibility to steer edge polaritons by means of grooves and nanocavities. The observed scattering of edge polaritons by defect structures is found to be in good agreement with finite-difference time-domain simulations. Our findings reveal the extraordinary capability of hyperbolic polariton propagation to cope with the presence of defects, providing an excellent basis for applications such as nanooptical circuitry, nanoscale cloaking and nanoscopic quantum technology.

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