Journal
POLYMER CHEMISTRY
Volume 12, Issue 2, Pages 183-188Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0py01545h
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Funding
- National Natural Science Foundation of China [21676057]
- Zhejiang Provincial Key Laboratory of Advanced Chemical Engineering Manufacture Technology [ACEMT-17-02]
- 111 Program of Fuzhou University
- Talent Program of Fuzhou University [GXRC-18041]
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An imine-based covalent organic framework, TFPPy-Td-COF, was synthesized and used as a catalyst for photo-induced controlled radical polymerization with copper under white light irradiation, leading to polymethylacrylates with narrow molecular weight dispersity and high chain-end fidelity. This new methodology opens up future possibilities for using robust and heterogeneous COF-based catalysts in CRP under visible light conditions.
An imine-based covalent organic framework, TFPPy-Td-COF, was synthesized to mediate photo-induced controlled radical polymerization (CRP) with copper under white light irradiation, providing polymethylacrylates with narrow molecular weight dispersity and high chain-end fidelity. This new methodology provides future directions for CRP using robust and heterogeneous COF-based catalysts under visible light conditions.
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