Journal
CHEMICAL COMMUNICATIONS
Volume 57, Issue 34, Pages 4130-4133Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d1cc01064f
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Inspired by the automated synthesis of DNA on a solid support, amphiphilic foldamers were synthesized from DAN and NDI building blocks, forming regular supramolecular nanotubes in water through donor/acceptor interactions and the solvophobic effect.
Inspired by the automated synthesis of DNA on a solid support, the electron-rich dialkoxynaphthalene (DAN) donor and the electron-deficient naphthalene-tetracarboxylic diimide (NDI) acceptor, amphiphilic foldamers have been synthesised from their respective phosphoramidite building blocks. The folding of the phosphodiester-linked hexamer (DAN-NDI)(3) revealed the formation of regular supramolecular nanotubes in water resulting from the self-assembly of multiple hexamers stabilized by donor/acceptor interactions and the solvophobic effect.
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