Journal
CHEMICAL COMMUNICATIONS
Volume 57, Issue 15, Pages 1895-1898Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0cc07119f
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Funding
- National Natural Science Foundation of China [21701007, 21801015]
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A general strategy based on host-guest interactions was used to fabricate atomically dispersed biomimetic catalysts, which have similar structure and function to enzymes, serving as active sites and reducing reaction activation energy.
Herein, we report a general strategy based on host-guest interactions to fabricate atomically dispersed biomimetic catalysts, which were evaluated by diboration of phenylacetylene. The structure and function of these mimics are quite similar to those of enzymes, namely, the atomically dispersed metal serves as an active site, the external macromolecular structure plays a role as an enzyme catalytic pocket to stabilize the reaction intermediates and the interactions between the intermediates and functional groups near to the active site can reduce the reaction activation energy.
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