4.6 Article

Water management by hierarchical structures for highly efficient solar water evaporation

Journal

JOURNAL OF MATERIALS CHEMISTRY A
Volume 9, Issue 11, Pages 7122-7128

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/d1ta00113b

Keywords

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Funding

  1. National Natural Science Foundation of China [21805004, 21671011, 21872001, 51801006]
  2. Beijing Municipal High Level Innovative Team Building Program [IDHT20180504]
  3. Beijing Outstanding Young Scientist Program [BJJWZYJH01201910005017]
  4. Beijing Natural Science Foundation [KZ201710005002, 2192005]
  5. Beijing Municipal Science and Natural Science Fund Project [KM201910005016]
  6. Beijing Postdoctoral Research Foundation [2020-ZZ-041]

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The study introduced the concept of water mass per unit surface area to regulate water management in devices and affect the evaporation rates. The optimized device utilizes different materials for water transportation, restriction, and photothermal functions, achieving high evaporation rates and energy efficiency.
Solar water evaporation is a sustainable and efficient way to produce fresh water. Identifying highly efficient photothermal materials is an important step for achieving high evaporation rates. However, the effects of the water interfacial area are rarely paid any attention, although a few reports have demonstrated high evaporation rates from micro-/nanostructured devices. In this work, we introduce a new term, water mass per unit surface area (WMUA), to connect the water mass and interfacial area. We can regulate WMUA using different commercial porous materials to realize water management in devices, which further affects the evaporation rates. The optimized device is composed of suedette sponge, filter paper, and polydopamine as the water-transportation, water-restrictive, and photothermal materials, respectively, and it achieves an evaporation rate of 1.8 kg m(-2) h(-1) and energy efficiency of similar to 92%. This presents a new strategy for the rational design of device structures and the promotion of evaporation rates, pushing this field into new areas.

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