Journal
DALTON TRANSACTIONS
Volume 50, Issue 2, Pages 490-493Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d0dt02709j
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Funding
- National Key Research and Development Program of China [2018YFA0208600]
- National Natural Science Foundation of China [21773242, 21935010]
- Youth Innovation Promotion of CAS [2016276]
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The new Cu(I) based boron imidazolate framework, BIF-105, exhibited efficient photocatalytic performance for CO2 reduction with high selectivity for CO under visible light irradiation.
A new Cu(i) based boron imidazolate framework, Cu[BH(im)(3)] (BIF-105, im = imidazole), with a two-dimensional fes-type layer structure was designed and synthesized. The resulting BIF-105 exhibited efficient photocatalytic performance for CO2 reduction with an evolution rate of 933 mu mol g(-1) h(-1) and a selectivity of 83.4% for CO under visible light irradiation, with [Ru(bpy)(3)]Cl-2 as the light absorber and triethanolamine as a sacrificial agent.
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