4.8 Review

High-entropy energy materials: challenges and new opportunities

Journal

ENERGY & ENVIRONMENTAL SCIENCE
Volume 14, Issue 5, Pages 2883-2905

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/d1ee00505g

Keywords

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Funding

  1. Helmholtz Association
  2. German Research Foundation [BR 3499/5-1, SE 1407/4-2, HA 1344/43-1]
  3. Kera-Solar project by Carl Zeiss Foundation
  4. EnABLES project - European Union [730957]
  5. EPISTORE project - European Union [101017709]

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The essential demand for functional materials enabling the realization of new energy technologies has driven significant efforts in scientific and industrial research. High-entropy materials, with their unique structural characteristics and tunable functional properties, have gained increasing interest in the fields of environmental science and renewable energy technology. Effective strategies for designing high-entropy materials from computational techniques and experimental aspects provide researchers with guidance on potential advantages and remaining challenges.
The essential demand for functional materials enabling the realization of new energy technologies has triggered tremendous efforts in scientific and industrial research in recent years. Recently, high-entropy materials, with their unique structural characteristics, tailorable chemical composition and correspondingly tunable functional properties, have drawn increasing interest in the fields of environmental science and renewable energy technology. Herein, we provide a comprehensive review of this new class of materials in the energy field. We begin with discussions on the latest reports on the applications of high-entropy materials, including alloys, oxides and other entropy-stabilized compounds and composites, in various energy storage and conversion systems. In addition, we describe effective strategies for rationally designing high-entropy materials from computational techniques and experimental aspects. Based on this overview, we subsequently present the fundamental insights and give a summary of their potential advantages and remaining challenges, which will ideally provide researchers with some general guides and principles for the investigation and development of advanced high-entropy materials.

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