4.7 Article

Self-cyclization vs. dimerization of o-alkenyl arylisocyanides: chemodivergent synthesis of quinolines and pyrrolo-fused diindoles

Journal

ORGANIC CHEMISTRY FRONTIERS
Volume 8, Issue 11, Pages 2595-2600

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/d1qo00132a

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Funding

  1. National Natural Science Foun-dation of China [21672034, 22001151]
  2. Taishan Scholar Program of Shandong Province
  3. Shandong Provincial Natural Science Foundation [ZR2019QB004]
  4. Large Instrument Open Foundation of Shandong Normal University [KFJJ2019003]

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A new method for solvent-dependent chemoselective Morita-Baylis-Hillman-type self-cyclization and dimerization of o-alkenyl arylisocyanides was developed, providing concise access to various 3-acylquinoline and pyrrolo[1,2-a:3,4-b ']diindole frameworks via distinct domino processes from the same starting materials.
Solvent-dependent chemoselective Morita-Baylis-Hillman-type self-cyclization and dimerization of o-alkenyl arylisocyanides were developed. These chemodivergent reactions provide concise access to the efficient synthesis of various 3-acylquinoline and pyrrolo[1,2-a:3,4-b ']diindole frameworks via the distinct domino process from the same starting materials.

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