4.7 Review

Recent developments of nanocarbon based supports for PEMFCs electrocatalysts

Journal

CHINESE JOURNAL OF CATALYSIS
Volume 42, Issue 8, Pages 1297-1326

Publisher

SCIENCE PRESS
DOI: 10.1016/S1872-2067(20)63736-6

Keywords

Nanocarbon support; Proton exchange membrane fuel cell; Electrocatalyst; Oxygen reduction reaction; Methanol oxidation reaction

Funding

  1. National Natural Science Foundation of China [21978331, 21975292, 21905311]
  2. Guangdong Basic and Applied Basic Research Foundation [2020A1515010343]
  3. Tip-top Scientific and Technical Innovative Youth Talents of Guangdong Special Support Program [2016TQ03N322]
  4. Guangzhou Science and Technology Project [201707010079]
  5. National Key Research and Development Program of China [2016YFB0101200]
  6. fundamental Research Funds for Central Universities [19lgpy136, 19lgpy116]
  7. China Postdoctoral Science Foundation [2019M653142]

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This paper provides an overview of the nanoarchitectures and surface physicochemical properties of nanocarbons affecting electrocatalyst performance, with discussions on recent progress in nanocarbon supports and guidance for future research directions.
Nanocarbons, widely and commonly used as supports for supported Pt-based electrocatalysts in PEMFCs, play a significant role in Pt dispersion and accessibility, further determining their corresponding electrocatalytic performance. This paper provides an overview of the nanoarchitectures and surface physicochemical properties of nanocarbons affecting the electrocatalyst performance, with an emphasis on both physical characteristics, including pore structure, and chemical properties, including heteroatom doping and functional carbon-based supports. This review discusses the recent progress in nanocarbon supports, guides the future development direction of PEMFC supports, and provides our own viewpoints for the future research and design of PEMFCs catalysts, advancing the commercialization of PEMFCs. (C) 2021, Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. All rights reserved.

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