4.6 Article

Droplet detachment and pinch-off of bidisperse particulate suspensions

Journal

SOFT MATTER
Volume 17, Issue 25, Pages 6202-6211

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/d1sm00593f

Keywords

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Funding

  1. National Science Foundation under NSF CAREER Program Award CBET Grant [1944844]
  2. ACS Petroleum Research Fund [60108-DNI9]
  3. Div Of Chem, Bioeng, Env, & Transp Sys
  4. Directorate For Engineering [1944844] Funding Source: National Science Foundation

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This paper experimentally investigates the thinning and pinch-off process of droplets in particle suspensions, showing that a bidisperse particle size distribution can lower viscosity and accelerate droplet formation. This result can be used to predict the dynamics of droplet formation with bidisperse suspensions.
When a droplet is generated, the ligament connecting the drop to the nozzle thins down and eventually pinches off. Adding solid particles to the liquid phase leads to a more complex dynamic, notably by increasing the shear viscosity. Moreover, it introduces an additional length scale to the system, the diameter of the particles, which eventually becomes comparable to the diameter of the ligament. In this paper, we experimentally investigate the thinning and pinch-off of drops of suspensions with two different sizes of particles. We characterize the thinning for different particle size ratios and different proportions of small particles. Long before the pinch-off, the thinning rate is that of an equivalent liquid whose viscosity is that of the suspension. Later, when the ligament thickness approaches the size of the large particles, the thinning accelerates and leads to an early pinch-off. We explain how the bidisperse particle size distribution lowers the viscosity by making the packing more efficient, which speeds up the thinning. This result can be used to predict the dynamics of droplet formation with bidisperse suspensions.

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