Journal
CHEMICAL COMMUNICATIONS
Volume 57, Issue 54, Pages 6672-6675Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d1cc02493k
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Funding
- Japan Society for the Promotion of Science (JSPS) [JP17K14483, JP19K05454, JP21K05067]
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A base-promoted switchable synthesis of five- and six-membered cyclic carbamates using atmospheric pressure carbon dioxide as the C1 source was developed. The chemoselectivity of products was controlled by changing bases and solvents. Experimental results and DFT studies revealed the reaction mechanism.
The base-promoted switchable synthesis of five- and six-membered cyclic carbamates using atmospheric pressure carbon dioxide as the C1 source was developed. The chemoselectivity of products was simply controlled by changing bases and solvents. The reaction proceeds effectively under mild conditions, affording valuable cyclic carbamates. Experimental results and DFT studies revealed the reaction mechanism.
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