4.6 Review

Mechanism of surface and interface engineering under diverse dimensional combinations: the construction of efficient nanostructured MXene-based photocatalysts

Journal

CATALYSIS SCIENCE & TECHNOLOGY
Volume 11, Issue 15, Pages 5028-5049

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/d1cy00803j

Keywords

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Funding

  1. National Natural Science Foundation of China [21607034]
  2. Beijing Natural Science Foundation [8192011]
  3. Science and Technology General Project of Beijing Municipal Education Commission [KM202010016006]
  4. Pyramid Talent Training Project of Beijing University of Civil Engineering and Architecture [JDYC20200313]
  5. National Key R&D Program of China [2020YFC1808805]
  6. Strategic Priority Research Program of the Chinese Academy of Sciences [XDB17000000]

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This review systematically summarizes the action principles of surfaces and interfaces in MXene-based photocatalysts, highlighting the impact of spatial conditions on surface and interface engineering. Furthermore, it discusses the advantages and challenges of the research direction of MXenes and MXene-based photocatalysts in the future.
As an emerging and growing family of two-dimensional transition metal carbides, carbonitrides, and nitrides, MXenes have received increasingly close attention due to their intriguing surface features, excellent electrical conductivity, and layered structures. The spatial conditions ascribed by the nanostructure of MXene-based photocatalysts are the decisive factor for their surface and interface characteristics, which play a vital role in expanding the light response range and inhibiting the recombination of photoinduced carriers. Although some reviews focus on the properties, synthesis strategies, and applications of MXene-based photocatalysts, there is still a lack of a comprehensive review that can provide the basis for MXene-based photocatalysts from the perspective of spatial conditions created by various nanostructures. In this review, we systemically summarize the action principles of surfaces and interfaces in MXene-based photocatalysts and highlight the impact of spatial conditions on surface and interface engineering by analyzing recent research on MXene-based photocatalysts. Furthermore, we put forward the advantages and challenges of the research direction of MXenes and MXene-based photocatalysts in the future.

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