4.3 Article

The Photodetectors Based on Lateral Monolayer MoS2/WS2 Heterojunctions

Journal

NANOSCALE RESEARCH LETTERS
Volume 16, Issue 1, Pages -

Publisher

SPRINGER
DOI: 10.1186/s11671-021-03581-4

Keywords

Lateral monolayer heterostructure; MoS2/WS2 heterojunction; Photodetector; Sharp interface

Funding

  1. National Natural Science Foundation of China [G0562011530131]
  2. National Key Research and Development Program of China [2019YFB2203400]
  3. 111 Project'' [B20030]
  4. UESTC Shared Research Facilities of Electromagnetic Wave and Matter Interaction [Y0301901290100201]
  5. Fundamental Research Funds for the Central Universities [ZYGX2019Z018]
  6. International Postdoctoral Exchange Fellowship Program (Talent-Introduction Program), China Postdoctoral Science Foundation [244125]
  7. Innovation Group Project of Sichuan Province [20CXTD0090]

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The study successfully synthesized large-area and high-quality lateral monolayer MoS2/WS2 heterojunctions, demonstrating their excellent performance. Photodetectors enhanced by the photogating effect exhibit competitive performance, but the 1/f noise from charge carrier trapping/detrapping hinders the development of the devices.
Monolayer transition metal dichalcogenides (TMDs) show promising potential for next-generation optoelectronics due to excellent light capturing and photodetection capabilities. Photodetectors, as important components of sensing, imaging and communication systems, are able to perceive and convert optical signals to electrical signals. Herein, the large-area and high-quality lateral monolayer MoS2/WS2 heterojunctions were synthesized via the one-step liquid-phase chemical vapor deposition approach. Systematic characterization measurements have verified good uniformity and sharp interfaces of the channel materials. As a result, the photodetectors enhanced by the photogating effect can deliver competitive performance, including responsivity of similar to 567.6 A/W and detectivity of similar to 7.17 x 10(11) Jones. In addition, the 1/f noise obtained from the current power spectrum is not conductive to the development of photodetectors, which is considered as originating from charge carrier trapping/detrapping. Therefore, this work may contribute to efficient optoelectronic devices based on lateral monolayer TMD heterostructures.

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