Journal
DALTON TRANSACTIONS
Volume 50, Issue 34, Pages 11711-11715Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d1dt02001c
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Funding
- National Natural Science Foundation of China [22078371, 21938001, 21961160741]
- Guangdong Provincial Key RD Programme [2019B110206002]
- Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program [2017BT01C102]
- NSF of Guangdong Province [2020A1515011141]
- National Key Research and Development Program Nanotechnology Specific Project [2020YFA0210900]
- Science and Technology Key Project of Guangdong Province, China [2020B010188002]
- Guangdong Basic and Applied Basic Research Foundation [2020A1515110864]
- Special fund for Local Science and Technology Development by the Central Government
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Atomically dispersed Fe species embedded in nitrogen-containing carbon supports (Fe-1/NC) are successfully synthesized using a ball milling approach with commercial protein powder as the nitrogen source. The catalyst exhibits outstanding performance in the oxidation of aromatic compounds containing saturated C-H bonds into corresponding ketones under ambient conditions, surpassing nanoparticle catalyst (Fe-n/NC) and metal-free catalyst (NC).
Atomically dispersed Fe species embedded in the nitrogen-containing carbon supports (Fe-1/NC) are successfully synthesized using a ball milling approach, with commercial protein powder as the nitrogen source. The catalyst exhibits outstanding performance in the oxidation of aromatic compounds containing saturated C-H bonds into corresponding ketones under ambient conditions, which is superior to those of a nanoparticle catalyst (Fe-n/NC) and a metal-free catalyst (NC).
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