Journal
EUROPEAN JOURNAL OF ORGANIC CHEMISTRY
Volume 2017, Issue 15, Pages 2118-2121Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ejoc.201601571
Keywords
Photoredox catalysis; Nickel; Cross-coupling; Radical reactions; C-C coupling
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Funding
- Centre National de la Recherche Scientifique (CNRS)
- Universite Pierre et Marie Curie (UPMC)
- Institut Universitaire de France (IUF)
- MSER (ASN PhD grant)
- LABEX MiChem [ANR-11-IDEX-0004-02]
- La Region Martinique (PhD grant)
- ANR NHCX [11-BS07-008]
- COST Action [CM1201]
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Alkylsilicates were engaged under photoredox/nickel dual catalysis conditions with alkyl halides for the first time. The C(sp(3))-C(sp(3)) cross-coupling products were obtained in moderate yields and were accompanied by the homocoupling products of the alkyl halide derivatives. These promising findings are strongly suggestive of the high synthetic potential of the dual catalytic approach for the forging of alkyl carbon-carbon bonds.
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