4.7 Article

Highly sensitive piezoresistive pressure sensors based on laser-induced graphene with molybdenum disulfide nanoparticles

Journal

SCIENCE CHINA-TECHNOLOGICAL SCIENCES
Volume 64, Issue 11, Pages 2408-2414

Publisher

SCIENCE PRESS
DOI: 10.1007/s11431-021-1899-9

Keywords

piezoresistive pressure sensor; laser-induced graphene foam; molybdenum disulfide nanoparticles; health monitoring

Funding

  1. Joint Doctoral Training Foundation of HEBUT
  2. National Natural Science Foundation of China [ECCS-1933072]
  3. National Heart, Lung, and Blood Institute of the National Institutes of Health [R61HL154215]
  4. Penn State University (Center for Security Research and Education)
  5. Penn State University (Center for Biodevices)
  6. Penn State University (College of Engineering)

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A flexible piezoresistive pressure sensor assembled with two 3D laser-induced graphene foam electrodes shows promising potential for low-cost, large-scale production and favorable sensing performance in motion detection and wrist pulse monitoring. Enhancement with MoS2 nanoparticles further increases sensitivity and sensing range, outperforming previous literature reports, while maintaining fast response/recovery rates and excellent durability/repeatability.
Wearable pressure sensors have drawn significant attention because of their extensive applications in motion detection, tactile sensing, and health monitoring. However, the complex manufacturing process and high cost of active materials make low-cost, large-scale production elusive. In this work, we report a flexible piezoresistive pressure sensor assembled with two 3D laser-induced graphene (LIG) foam electrodes on a polyimide thin film from a simple laser scribing process in the ambient environment. The design of the air gap between the two foam electrodes allows the sensor to showcase a low limit of detection of 0.274 Pa, which provides favorable sensing performance in motion detection and wrist pulse monitoring. The addition of spherical MoS2 nanoparticles between the two foam electrodes further enhances the sensitivity to 88 kPa(-1) and increases the sensing range to significantly outperform the previous literature reports. The demonstrated LIG pressure sensors also exhibit fast response/recovery rates and excellent durability/repeatability.

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