Journal
CHEMICAL COMMUNICATIONS
Volume 57, Issue 87, Pages 11505-11508Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d1cc05491k
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Funding
- Baden-Wurttemberg Stiftung [3443]
- Panamanian National System of Investigators (SNI, SENACYT)
- DFG [FE 1776/2-1, WE 1863/34-1]
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The FID-detected nutations of the antiferromagnetic crystal [Y(pc)(2)] show that its radical spin can be driven coherently in its magnetically condensed undeuterated phase at room temperature. In liquid-helium measurements, additional Rabi oscillations were observed, attributed to transitions within higher-multiplicity states of finite-sized chain fragments.
FID-detected nutations of the antiferromagnetic crystal form of [Y(pc)(2)] demonstrated that its radical spin can be coherently driven in its magnetically condensed undeuterated phase and at room temperature. Liquid-helium nutations revealed additional Rabi oscillations assigned to transitions within higher-multiplicity states of finite-sized chain fragments.
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