Journal
ESCIENCE
Volume 1, Issue 1, Pages 28-43Publisher
KEAI PUBLISHING LTD
DOI: 10.1016/j.esci.2021.10.001
Keywords
Calixarene; Electrochemistry; Energy Storage; Pillararene; Theoretical Simulations
Funding
- Young Talent Support Plan of Xi'an Jiaotong University [010600-11301291010702, 010600-71211201010715, 050700-71240000000046]
- Natural Science Foundation of Shaanxi Province [2021JM-006]
- National Natural Science Foundation of China [62074123, 61701543]
- PetroChina Innovation Foundation [2019D-5007-0410]
- Singapore National Research Foundation Investigator Ship [NRF-NRFI2018-03]
- Singapore Academic Research Fund [TR12/19]
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This review discusses the current advances in developing electrochemical energy materials based on pillararene/calixarene systems, covering fundamental mechanisms, simulation studies, and practical applications, with a focus on their use in lithium/sodium-ion batteries and supercapacitors. The diverse roles and design strategies for high-performance pillararene/calixarene-based batteries are analyzed, along with prospects for further developments in this emerging field. Overall, the review provides a comprehensive overview of the unique properties and applications of pillararene/calixarene-based materials in electrochemical energy storage devices.
Pillararene/calixarene-based functional materials have garnered significant attention for their unique topological/chemical structures and physicochemical properties, and their extended applications in electro-chemistry have given rise to a promising area of research. This review details current advance in developing electrochemical energy materials based on pillararene/calixarene systems from the viewpoint of both fundamental theoretical simulations and research on practical applications. First, we discuss the underlying mechanisms of applying pillararene/calixarene-based systems for electrochemical energy applications. Second, we summarize simulation studies on pillarquinone and calixquinone with intrinsic structures for applications in batteries. In addition, state-of-the-art applications of pillararene/calixarene-based systems in electrochemical energy storage devices such as lithium/sodium-ion batteries and supercapacitors are highlighted. The diverse roles they play and the various design strategies that have been investigated for high-performance pillararene/calixarene-based batteries are analyzed. Finally, we discuss the prospects for further developments in this emerging field. This review not only describes recent advances in pillararene/calixarene-based batteries and supercapacitors but also lays a firm groundwork for their further application in electrochemical energy engineering.
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