Journal
ATMOSPHERIC CHEMISTRY AND PHYSICS
Volume 21, Issue 21, Pages 16575-16591Publisher
COPERNICUS GESELLSCHAFT MBH
DOI: 10.5194/acp-21-16575-2021
Keywords
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Funding
- French National Research Agency [ANR-15-CE01-0014-01]
- French national programme LEFE/INSU
- Programme National de Teledetection Spatiale (PNTS) [PNTS-2016-14]
- French National Agency for Space Studies (CNES)
- South African National Research Foundation (NRF) [UID 105958]
- European Union [312609]
- Atmospheric Research in Southern Africa and the Indian Ocean (AR-SAIO) project (CNRS)
- South African NRF
- PICS (CNRS) [260888]
- PHC PROTEA of the French Ministry of Foreign Affairs and International Development [33913SF, 38255ZE]
- Programme National de Teledetection Spatiale [PNTS-2016-14]
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This study presents the first objective classification of the synoptic variability controlling the spatial distribution of BBA in southern Africa and the South Atlantic during austral winter. By analysing atmospheric circulation data, a six-class weather regime classification is constructed, revealing the influence of midlatitude disturbances and pressure anomalies in the South Atlantic on BBA transport towards southern extratropics. The results show the potential for using the weather regime classification as a diagnostic tool for aerosol dynamics and understanding complex radiation-aerosol-cloud interactions in the region.
During austral winter, a compact low cloud deck over the South Atlantic contrasts with clear sky over southern Africa, where forest fires triggered by dry conditions emit large amounts of biomass burning aerosols (BBAs) in the free troposphere. Most of the BBA burden crosses the South Atlantic embedded in the tropical easterly flow. However, midlatitude synoptic disturbances can deflect part of the aerosol from the main transport path towards southern extra-tropics. In this study, the first objective classification of the synoptic variability controlling the spatial distribution of BBA in southern Africa and the South Atlantic during austral winter (August to October) is presented. By analysing atmospheric circulation data from reanalysis products, a six-class weather regime (WR) classification of the region is constructed. The classification reveals that the synoptic variability is composed of four WRs, representing disturbances travelling at midlatitudes, and two WRs accounting for pressure anomalies in the South Atlantic. The WR classification is then successfully used to characterise the aerosol spatial distribution in the region in the period 2003-2017, in both reanalysis products and station data. Results show that the BBA transport towards southern extratropics is controlled by weather regimes associated with midlatitude synoptic disturbances. In particular, depending on the relative position of the pressure anomalies along the midlatitude westerly flow, the BBA transport is deflected from the main tropical route towards southern Africa or the South Atlantic. Moreover, the WRs accounting for midlatitude disturbances show organised transition sequences, which allow one to illustrate the evolution of the BBA northerly transport across the region in the context of a wave pattern. The skill in characterising the BBA transport shown by the WR classification indicates the potential for using it as a diagnostic/predictive tool for the aerosol dynamics, which is a key component for the full understanding and modelling of the complex radiation-aerosol-cloud interactions controlling the atmospheric radiative budget in the region.
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