Journal
SMALL SCIENCE
Volume 1, Issue 12, Pages -Publisher
WILEY
DOI: 10.1002/smsc.202100015
Keywords
CO2 reduction; electrocatalysis; host-guest composites; hydrogen oxidation; metal-organic frameworks; oxygen reduction; water splitting
Funding
- Strategic Priority Research Program of the Chinese Academy of Sciences [XDA09040100]
- National Key Basic Research Program of China [2016YFA0200700]
- Frontier Science Key Project of the Chinese Academy of Sciences [QYZDJ-SSW-SLH038]
- National Natural Science Foundation of China [21890381, 21721002]
- K.C. Wong Education Foundation
- FH Loxton fellowship of the USYD
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Metal-organic frameworks (MOFs) are a new family of catalytic materials with unique physicochemical properties, attracting extensive attention in the field of electrocatalysis. Significant advancements have been made in creating pristine MOF-based materials for important energy conversions.
Electrocatalysis is at the heart of many significant chemical transformation processes and advanced clean energy technologies. Traditional noble/transition metal oxides are widely used as electrocatalysts; however, they often suffer from intrinsic disadvantages, including low atom utilization, small surface area, and unfavorable tunability. Metal-organic frameworks (MOFs), as a new family of catalytic materials, are attracting extensive attention due to their unique physicochemical properties. The tremendous pristine MOF-based materials are created using various synthetic approaches and further used for important energy conversions. Herein, a systematic overview on the unique merits and the state-of-the-art design of MOF-based electrocatalysts is offered. This review also presents recent advances in the development of various pristine MOFs and MOF-based host-guest composite catalysts for electrocatalysis (i.e., oxygen reduction reaction, hydrogen oxidation reaction, hydrogen evolution reaction, oxygen evolution reaction, and CO2 reduction reaction) and discusses the future challenges and opportunities in this emerging field.
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