Unidirectional emission of phase-controlled second harmonic generation from a plasmonic nanoantenna

Shaping the emission pattern of second harmonic (SH) generation from plasmonic nanoparticles is important for practical applications in nonlinear nanophotonics but is rendered challenging by the complex second-order nonlinear-optical processes. Here, we theoretically and experimentally demonstrate that a pair of V and Y-shaped gold nanoparticles directs the SH emission perpendicularly to an incident light direction. Owing to spatial overlap of two orthogonal plasmonic dipole modes at the fundamental and SH wavelengths of the individual particles, surface SH polarizations induced by the fundamental field is efficiently near-field coupled to the SH plasmon mode, resulting in dipolar SH emission from the individual particles. Moreover, the phase of this emission can be tuned simply by altering the part of the Y-particle shape, which changes the SH plasmon resonance while keeping the fundamental resonance. Our approach is a promising platform for engineering not only directional nonlinear nanoantennas but also nonlinear metamaterials.

Automated summary

A pair of V and Y-shaped gold nanoparticles are able to emit second harmonic (SH) radiation perpendicularly to the incident light direction, and the phase of this emission can be modulated by altering the shape of the Y-particle. This approach can be used to engineer directional nonlinear nanoantennas and nonlinear metamaterials.