Journal
ENERGY & ENVIRONMENTAL SCIENCE
Volume 10, Issue 4, Pages 893-899Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6ee03145e
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Funding
- Natural Science Foundation of China [51573214, 21573066]
- Youth 1000 Talent Program of China
- National Key Research and Development Program of China [2016YFB0302301]
- National Postdoctoral Program for Innovative Talents [BX201600195]
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A general and effective approach was proposed to fabricate a new family of Co-based bimetallic phosphide ultrathin nanosheets (CoM-P-NS, M = Ni, Mn, Cu, Zn) with homogeneous composition and unique porous architecture using ultrathin metal-organic framework nanosheets (MOFNs) as precursors for the first time, which yielded synergistically active sites, mass transport and dynamic modulations for the oxygen evolution reaction (OER). The optimized samples showed remarkable oxygen evolution activity in alkaline electrolytes, outperforming both the commercial RuO2 and Ir/C benchmarks and ranking the best among all the metal-phosphide electrocatalysts reported to date.
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