Journal
ENERGIES
Volume 10, Issue 7, Pages -Publisher
MDPI AG
DOI: 10.3390/en10070961
Keywords
photoflash exposure; nascent soot particles; nanostructure; oxidation reactivity
Categories
Funding
- National Natural Science Foundation of China [51576100, 51506095]
- Jiangsu Provincial Natural Science Foundation of China [BK20140034]
- Jiangsu Provincial Innovative Project of Graduate Education [KYZZ16_0184]
- Jiangsu Provincial Project of Six Talent Summit [2014-XNY-002, 2015-XNY-004]
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Soot particles are a kind of major pollutant from fuel combustion. To enrich the understanding of soot, this work focuses on investigating detailed influences of instantaneous external irradiation (conventional photoflash exposure) on nanostructure as well as oxidation reactivity of nascent soot particles. By detailed soot characterizations flash can reduce the mass of soot and soot nanostructure can be reconstructed substantially without burning. After flash, the degree of soot crystallization increases while the soot reactive rate decreases and the activation energy increases. In addition, nanostructure and oxidative reactivity of soot in air and Ar after flash are different due to their different thermal conductivities.
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