Journal
CHEMICAL SOCIETY REVIEWS
Volume 51, Issue 6, Pages 1881-1898Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d1cs01171e
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Funding
- Australian Research Council (A.L.C. Fellowship) [DE200100450]
- Australian National University Futures Scheme
- Australian Research Council [DE200100450] Funding Source: Australian Research Council
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This article examines modes of cooperativity and catalytic mechanisms in metal-metal cooperative catalysts by studying (de)hydrogenation processes and drawing lessons from the development of metal-ligand cooperative catalysts.
Metal-ligand cooperativity (MLC) is an established strategy for developing effective hydrogenation and dehydrogenation catalysts. Metal-metal cooperativity (MMC) in bimetallic complexes is not as well understood, and to date has had limited implementation in (de)hydrogenation. Herein we use (de)hydrogenation processes as a platform to examine modes of cooperativity, with a particular focus on catalytic mechanisms. We investigate how lessons learnt from the extensive development of metal-ligand cooperative catalysts can aid the ongoing development of metal-metal cooperative catalysts.
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