Journal
CHEMICAL COMMUNICATIONS
Volume 58, Issue 34, Pages 5229-5232Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d2cc00657j
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Funding
- KAKENHI [17H06444, 19H00903, 20K21209]
- Japan Society for the Promotion of Science [15H05480, 17K19185, 17H05391, 19H04602, 19H05777, 20H02754, 20K15955]
- JST PRESTO [JPMJPR20A4]
- JST CREST, Japan [JPMJCR20B6]
- Iketani Science and Technology Foundation
- Izumi Science and Technology Foundation
- Mazda Foundation
- Grants-in-Aid for Scientific Research [20H02754, 19H04602, 20K15955, 19H05777, 20K21209, 17H05391, 17K19185, 17H06444, 19H00903] Funding Source: KAKEN
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A new Ru polypyridyl complex with an N-heterocyclic carbene ligand was synthesized and characterized in this study. The complex exhibited strong absorption in the visible-light region due to the electron-donating nature of the carbene ligand, and showed efficient catalytic activity for visible light-driven CO2 reduction, with a reaction rate of 36.7 h(-1).
A novel Ru polypyridyl complex with an N-heterocyclic carbene ligand was successfully synthesised and characterised. The complex exhibited an intense absorption band in the visible-light region derived from the strong electron-donating character of the carbene ligand, and efficiently catalysed the visible light-driven CO2 reduction with the reaction rate of 36.7 h(-1).
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