Journal
ADVANCED ENERGY AND SUSTAINABILITY RESEARCH
Volume 3, Issue 7, Pages -Publisher
WILEY
DOI: 10.1002/aesr.202200004
Keywords
CO2 reduction; metal-organic frameworks; photocatalysis; structure designs
Categories
Funding
- National Key R&D Program of China [2021YFA1500402]
- National Natural Science Foundation of China (NSFC) [22105203, 22175174]
- Natural Science Foundation of Fujian Province [2020J01116, 2021J06033]
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In this review, the recent progress in the rational design and performance enhancement of metal-organic framework (MOF)-based photocatalysts for CO2 reduction is summarized, and the current pending issues and future development prospects are discussed.
Photocatalytic carbon dioxide (CO2) reduction can utilize solar light to convert CO2 to high value-added products, which thus are recognized as an intriguing strategy to solve excessive CO2 emissions. Metal-organic framework (MOF)-based photocatalysts have shown high potential in the field of CO2 reduction due to their high porosity and tunable structure. In this review, the recent progress achieved in the rational design of MOF-based photocatalysts, including the pure MOF materials, MOF-based composites, and the derivatives of MOFs, for the reduction of CO2, are summarized and the developed modification strategies to enhance the photocatalytic performance of MOF-based photocatalysts are highlighted. The current pending issues and the outlook for the future development are also discussed.
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