4.8 Article

Plasmonic crescent nanoarray-based surface lattice resonance sensor with a high figure of merit

Journal

NANOSCALE
Volume 14, Issue 16, Pages 6144-6151

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/d1nr08341d

Keywords

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Funding

  1. National Key R&D Program of China [2019YFC1708704, 2019YFC1708701]
  2. National Natural Science Foundation of China [62073068, 62073061]
  3. Fundamental Research Funds for the Central Universities [N180402023]
  4. Liaoning Revitalization Talents Program [XLYC1907016]
  5. Science and Technology Project of Shenyang [20-206-4-20]
  6. Natural Science Foundation of Liaoning Province [2020-MS-077]
  7. Hebei Natural Science Foundation [F2020501040]
  8. Natural Science Foundation of Shandong Province [ZR2020MF108]
  9. Liaoning Province Key R&D Plan Guidance Project [2019JH8/10300109]

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A surface lattice resonance (SLR) sensor based on crescent nanoarrays is proposed in this work, which can achieve a high figure of merit (FOM) by adjusting the structural parameters of the arrays. Experimental results show that the FOM can reach a level higher than 1000 RIU-1, and this sensor demonstrates great potential in trace substance detection.
Due to the natural accumulation of radiation losses arising from the localization and random arrangement of nanoparticles, the figure of merit (FOM) of localized surface plasmon resonance (LSPR) sensors is usually very low (the value is usually less than 5 RIU-1). However, radiation losses of individual particles will be offset by adjusting the phase of the scattered field which is dependent on the structure parameters of arrays. Based on this, a two-dimensional periodic crescent nanoarray-based surface lattice resonance (SLR) sensor with a high FOM is proposed in this work. Some significant results have been obtained by mode field analysis and adjustment of structural parameters. On the one hand, the line-shape of the SLR spectrum is divided into a Fano-like line and a separate line. And the former usually has an FOM of 10(1) magnitude while the latter has an FOM of 10(3) magnitude. On the other hand, the relative size of the excitation wavelengths between SLR and LSPR is also vital. The FOM is higher but resonance depth decreases faster when the relative size increases. In this work, a full width at half-maximum (FWHM) of less than 0.5 nm and FOM of more than 1000 RIU-1 (the quality factor is more than 3000) are achieved by the proposed crescent nanoarrays. In addition, this structure demonstrates that plasmonic nanoarray-based SLR has enormous potential in trace substance detection.

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