Journal
FRONTIERS IN CHEMISTRY
Volume 4, Issue -, Pages -Publisher
FRONTIERS MEDIA SA
DOI: 10.3389/fchem.2016.00007
Keywords
CH4 adsorption; palladium; TAP reactor; metal/support interface; NGV catalyst
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Funding
- French Environment and Energy Management Agency (Ademe)
- North Region through the Institut de Recherche en Environnement Industriel (IRENI)
- National Agency for Research (ANR)
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Temporal Analysis of Products (TAP) investigation on Natural Gas-fueled Vehicle (NGV) catalysts provides information related to the nature of reaction steps involved over noble metals and at the metal-support interface. The determination of accurate kinetic parameters for methane adsorption from single pulse experiments and subsequent investigation of sequential surface reactions from alternative CH4/O-2 pulse experiments is the first step toward the establishment of relevant structure/activity relationships which can highlight the importance of the metal/support interface on freshly-prepared and aged single palladium based catalysts.
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