Journal
CATALYSIS SCIENCE & TECHNOLOGY
Volume 12, Issue 11, Pages 3431-3435Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d2cy00614f
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Funding
- National Natural Science Foundation of China [21971221, 21401162, 21773203]
- Yangzhou University Interdisciplinary Research Foundation for Chemistry Discipline of Targeted Support [yzuxk202010]
- Postgraduate Research & Practice Innovation Program of Jiangsu Province [XKYCX19_062]
- Fundamental Research Funds for the Central Universities [301918014103]
- High-Level Entrepreneurial and Innovative Talents Program of Jiangsu
- Lvyangjinfeng Talent Program of Yangzhou
- Priority Academic Program Development of Jiangsu Higher Education Institutions [12KJB150023]
- Top-notch Academic Programs Project of Jiangsu Higher Education Institutions [PPZY2015B112]
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Thiomolybdate clusters combined with mesoporous carbon spheres serve as sulfur host, increasing overall electrical conductivity through inner carbon capsule and enhancing the redox kinetics of polysulfides via bidirectional catalysis, thereby confining volume expansion of sulfur and shuttle effect.
Thiomolybdate [Mo3S13](2-) clusters combined with mesoporous carbon spheres are employed as sulfur host. Such structures not only increase overall electrical conductivity via inner carbon capsule, but also enhance the redox kinetics of polysulfides by the bidirectional catalysis of [Mo3S13](2-), thus confining the volume expansion of sulfur and shuttle effect.
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