Journal
ACS MATERIALS LETTERS
Volume 4, Issue 6, Pages 1025-1031Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsmaterialslett.2c00099
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Funding
- NSERC through the Alexander Graham Bell Canada Graduate Scholarship Doctoral Program
- Concordia University Research Chair program
- Natural Sciences and Engineering Research Council of Canada (NSERC) [DGECR-2018-00344, DG-2016-06655]
- Cette recherche a ete financee par le Conseil de recherches en sciences naturelles et en genie du Canada (CRSNG) [DGECR-2018-00344, DG-2016-06655]
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A facile route for modulating the photoluminescent and radioluminescent properties of Tb(III)-based MOFs is reported in this work, using Tb(III) cluster nodes as X-ray attenuators and organic linkers with varying excited state energies as sensitizers.
Luminescent metal-organic frameworks (MOFs) are of interest for sensing, theranostics, dosimetry, and other applications. The use of lanthanoids in MOF nodes allows for intrinsic metal-based luminescence. In this work, a facile route for modulating the photoluminescent and radioluminescent properties of Tb(III)-based MOFs is reported. By using Tb(III) cluster nodes as X-ray attenuators, and organic linkers with varying excited state energies as sensitizers, MOFs with metalbased, linker-based, and metal+linker-based photo- and radioluminescence are reported.
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