4.6 Article

Revealing intrinsic spin coupling in transition metal-doped graphene

Journal

PHYSICAL CHEMISTRY CHEMICAL PHYSICS
Volume 24, Issue 26, Pages 16300-16309

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/d2cp00906d

Keywords

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Funding

  1. National Natural Science Foundation of China [22073049, 22122303]
  2. Natural Science Foundation of Tianjin City [20JCQNJC01760]
  3. Fundamental Research Funds for the Central Universities (Nankai University) [63206008]

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This research comprehensively studies the spin couplings between transition metal atoms doped on graphene and reveals their potential application in spintronic device design. It also verifies that the spin-coupling effect can exhibit a certain distance dependence and space propagation.
Graphene materials offer attractive possibilities in spintronics due to their unique atomic and electronic structures, which is in contrast to their limited applications in the design of sophisticated spintronic devices. This should be attributed to the lack of knowledge about the intrinsic characteristics of graphene materials, especially the diverse correlations between sites within the materials and their roles in spin-signal generation and propagation. This work comprehensively studies the spin couplings between transition metal atoms doped on graphene and reveals their potential application in spintronic device design through the realization of various logic gates. In addition, the effects of the distance between doped metal atoms and the number of carbon layers on the logic gate implementation further verify that the spin-coupling effect can exhibit a certain distance dependence and space propagation. The achievements in this work uncover the potential value of graphene materials and are expected to open up new avenues for exploring their application in the design of sophisticated spintronic devices.

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