Journal
CATALYSIS SCIENCE & TECHNOLOGY
Volume 12, Issue 15, Pages 4851-4856Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d2cy00797e
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Funding
- National Key R&D Program of China [2017YFA0204701]
- Chinese Academy of Sciences [QYZDY-SSWSLH024]
- National Natural Science Foundation of China [22071256]
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Two highly crystalline coordination polymers, Pb-HBT and Pb-BDT, were synthesized and displayed high photocatalytic activities for the oxidation reactions of amines to imines under mild conditions.
Two highly crystalline coordination polymers (CPs), namely, Pb-HBT and Pb-BDT, were synthesized from the reaction of Pb(ii) ions with 4-hydroxybenzenethiol (HBT) and 1,4-benzenedithiol (BDT). Both of these CPs display similar layer structures of alternately stacked two-dimensional PbS networks and benzene units according to their crystal structures solved based on high resolution powder X-ray diffraction data. They exhibit high photocatalytic activities for the oxidation reactions of amines to imines under mild conditions, i.e., in air and at room temperature under sacrificial reagent-, co-catalyst- and redox mediator-free conditions.
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